Mainly for globtops, Ben and others did it for the Radica, so it has to be possible, just not sure the exact route to go about it (this is for a ~55 pin rom)
Current status here: http://nesdev.parodius.com/bbs/viewtopic.php?p=15095
Finding custom ROM pinouts
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I'm not sure how Ben found out about the pinout, I suspect he either just went with the assumption that it was a Genesis and wired it up from there, or had gotten the schematics from somewhere.
Other than just wiring it up in a logical manner for a NES cart, or getting the schematics, you could try getting ahold of a digital logic analyser with a bunch of channels (or use a single channel one on each of the pins) and watch the output.
Other than just wiring it up in a logical manner for a NES cart, or getting the schematics, you could try getting ahold of a digital logic analyser with a bunch of channels (or use a single channel one on each of the pins) and watch the output.